Solid-state and Solution Studies on a β-Diketiminate Zinc Hydride Complex

[MesnacnacZn(μ-H)]2 (1) was synthesized by reaction of MesnacnacZnI with either an equimolar amount of KNH(iPr)BH3 or an excess of NaH and characterized by multinuclear NMR and IR spectroscopy as well as X-ray diffraction. Two polymorphs of 1 were found and their structures determined on single crystals.

Dedicated to Professor Hubert Schmidbaur on the occasion of his 75th birthday.

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