If two solid particles collide, charge is exchanged. However, this transfer is not restricted to the surface of the particle. Ions are also dispersed into the environment. They form a charge cloud around the particle. In this way, all particle-laden atmospheres from volcanic plumes on Earth over exoplanet atmospheres to protoplanetary disks might be subject to gas-phase ionization by means of particle collisions. In laboratory experiments, we quantify the amount of ions produced in a collision of glass beads with 2.8 mm diameter. We extract the ions by applying an external electrostatic field and measuring the generated current. The ions are detected at all the pressures studied, i.e., from 0.3 mbar to 100 mbar. However, the ionization rate peaks at about 1 mbar. Scaled to individual bouncing collisions, charge as high as ∼1 pC of each polarity was detected. This implies collisions of grains can be a significant source of ions in various atmospheres.